• Intrinsic Z-DNA Is Stabilized by the Conformational Selection Mechanism of Z-DNA-Binding Proteins

    Sangsu Bae, Doyoun Kim, Kyeong Kyu Kim, Yang-Gyun Kim, Sungchul Hohng

    Journal of the American Chemical Society

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    https://doi.org/10.1021/ja107498y

    Abstract

    Z-DNA, a left-handed isoform of Watson and Crick’s B-DNA, is rarely formed without the help of high salt concentrations or negative supercoiling. However, Z-DNA-binding proteins can efficiently convert specific sequences of the B conformation into the Z conformation in relaxed DNA under physiological salt conditions. As in the case of many other specific interactions coupled…


  • Single-molecule four-color FRET

    Jinwoo Lee, Sanghwa Lee, Kaushik Ragunathan, Chirlmin Joo, Taekjip Ha, Sungchul Hohng

    Angewandte Chemie (International ed. in English)

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    https://doi.org/10.1002/anie.201005402

    Abstract

    Six interfluorophore FRET efficiencies Eij (see scheme) can be determined in real time by a single-molecule four-color FRET technique both in confocal and in total-internal-reflection fluorescence microscopy. This technique was used to probe the correlated motion of the four arms of the Holliday junction, and to assess correlation of RecA-mediated strand exchange events at both…

    Single-molecule four-color FRET

  • Single-Molecule Three-Color FRET with Both Negligible Spectral Overlap and Long Observation Time

    Sanghwa Lee, Jinwoo Lee, Sungchul Hohng

    Abstract

    Full understanding of complex biological interactions frequently requires multi-color detection capability in doing single-molecule fluorescence resonance energy transfer (FRET) experiments. Existing single-molecule three-color FRET techniques, however, suffer from severe photobleaching of Alexa 488, or its alternative dyes, and have been limitedly used for kinetics studies. In this work, we developed a single-molecule three-color FRET technique…


  • Highly Polymorphic G-quadruplexes in the c-MYC Promoter

    Jeong-Min Yoon, Hyun-Jin Kang, Jae-Ho Sung, Hyun-Ju Park, Sung-Chul Hohng

    Bulletin of the Korean Chemical Society

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    https://doi.org/10.5012/bkcs.2010.31.04.1025

    Abstract

    Guanine-rich tracts are frequently found in various regions of genomic DNA such as telomeres, centromeres, and promoters of proto-oncogenes, but rarely in the promoter of tumor-suppressor genes. When a G-tract has more than four G-stretches, it can form a G-quadruplex, a non-Watson-Crick DNA structure stabilized by a successive stacking of guanine tetrads. Guanine tetrad is…

    Highly Polymorphic G-quadruplexes in the c-MYC Promoter

  • Single-molecule FRET studies on frameshifting RNA structures of human immunodeficiency virus

    Hee-Sun Hong, Yang-Gyun Kim, Sung-Chul Hohng

    Bulletin of the Korean Chemical Society

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    https://doi.org/10.5012/bkcs.2010.31.04.1021

    Abstract

    Correspondence between DNA sequences and its protein product is not straightforward because the genetic information can be dynamically reprogrammed during various steps of genetic decoding process. The programmed -1 ribosomal frameshifting (-1PRF) is an example of such genetic recoding mechanisms, where the reading frame of the translation machinery is shifted toward -1 direction at a…